Just a little update.
Setting NetworkThrottlingIndex to FFFFFFFF actually disables the limiter entirely, but regardless, I've found no negative effects when it's disabled. I can still happily stream HD video over my LAN whilst copying files.
I'm yet to try enabling jumbo frames, but as they're disabled by default and this solution works, I'm going to leave things as they are.
Thanks to everyone who contributed data and ideas. It's great to finally have this solved.
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